Investigation of Synthesis and Deposition Methods for Cesium-Based Perovskite Quantum Dots for Solar Cell Applications
DOI:
https://doi.org/10.18321/ectj1437Keywords:
Perovskites, Quantum dots, Hot injection, Recycling, Deposition, Synthesis, Thin filmsAbstract
The CsPbI2Br perovskite quantum dots (PQDs) have great potential in photovoltaic applications due to their phase stability and optoelectronic properties. In this work, the synthesis technique of CsPbI2Br PQDs with the investigation of their properties and applications are identified. The critical issues and precautions for preparing PQDs are also discussed. It is also interesting to find that the collected supernatant solutions during the purification of PQDs can be recycled for preparing other types of PQDs. Meanwhile, this work demonstrates different approaches (i) thermal annealing, usage of (ii) methyl acetate and (iii) ethyl acetate as anti-solvents for preparing CsPbI2Br PQDs in the form of thin films on glass substrates. The obtained samples are characterized in terms of morphology, structural and optical properties. The results of this work can provide useful information for researchers, particularly for those who are starting to synthesize PQDs for fabrications of solid-state devices.
References
(1). F. Bella, P. Renzi, C. Cavallo, C. Gerbaldi, Chem.- Eur. J. 24 (2018). 12183‒12205. Crossref
(2). W. Chen, X. Li, Y. Li, Y. Li, Energy Environ. Sci. 13 (2020) 1971‒1996. Crossref
(3). W. Chi, S.K. Banerjee, Small 16 (2020) 1907531. Crossref
(4). C. Lee, Y. Shin, G.G. Jeon, D. Kang, et al., Energies 14 (2021) 201. Crossref
(5). Z. Qiu, N. Li, Z. Huang, Q. Chen, et al., Small Methods 4 (2020) 1900877. Crossref
(6). L. Liu, A. Najar, K. Wang, M. Du, et al., Adv. Sci. 9 (2022) 2104577. Crossref
(7). R. Syah, A. Davarpanah, M.K.M. Nasution, Q. Wali, et al., Coatings 11 (2021) 1173. Crossref
(8). E.A. Erazo, H.E. Sánchez-Godoy, A.F. Gualdrón- Reyes, S. Masi, et al., Nanomaterials 10 (2020) 1586. Crossref
(9). C. Liu, M. Hu, X. Zhou, J. Wu, et al., NPG Asia Mater. 10 (2018) 552–561. Crossref
(10). NREL, Https://Www.Nrel.Gov/Pv/Cell-Efficiency. Html, Best Research-Cell Efficiency Chart (2022).
(11). H. Li, T. Luo, S. Zhang, Z. Sun, et al., Energy and Environmental Materials 4 (2021) 46‒64. Crossref
(12). W. Chi, S.K. Banerjee, Angew. Chem. 134 (2022) e202112412. Crossref
(13). R.X. Yang, L.Z. Tan, J. Chem. Phys. 152 (2020) 034702. Crossref
(14). J. Chen, D. Jia, E.M.J. Johansson, A. Hagfeldt, et al., Energy Environ. Sci. 14 (2021) 224‒261. Crossref
(15). B. Chaudhary, Y.K. Kshetri, H.S. Kim, S.W. Lee, et al., Nanotechnology 32 (2021). Crossref
(16). L. Protesescu, S. Yakunin, M.I. Bodnarchuk, F. Krieg, et al., Nano Lett. 15 (2015) 3692–3696. Crossref
(17). H. Wang, H. Bian, Z. Jin, H. Zhang, et al., Chem. Mater. 31 (2019) 6231–6238. Crossref
(18). J. Kim, S. Cho, F. Dinic, J. Choi, et al., Nano Energy 75 (2020) 104985. Crossref
(19). Y. Wang, J. Yuan, X. Zhang, X. Ling, et al., Adv. Mater. 32 (2020) 2000449. Crossref
(20). R. Han, Q. Zhao, J. Su, X. Zhou, et al., J. Phys. Chem. C 125 (2021) 8469–8478. Crossref
(21). X. Zhang, H.C. Wang, A.C. Tang, S.Y. Lin, et al., Chem. Mater. 28 (2016) 8493–8497. Crossref
(22). H. Huang, L. Polavarapu, J.A. Sichert, A.S. Susha, et al., NPG Asia Mater. 8 (2016). Crossref
(23). C.J. Thomas, Y. Zhang, A. Guillaussier, K. Bdeir, et al., Chem. Mater. 31 (2019) 9750–9758. Crossref
(24). R. An, F. Zhang, X. Zou, Y. Tang, et al., ACS Appl. Mater. Interfaces 10 (2018) 39222–39227. Crossref
(25). Y. Li, X. Wang, W. Xue, W. Wang, et al., Nano Res. 12 (2019) 785–789. Crossref
(26). Q. Zeng, X. Zhang, C. Liu, T. Feng, et al., Solar RRL 3 (2019) 1800239. Crossref
(27). A. Swarnkar, A.R. Marshall, E.M. Sanehira, B.D. Chernomordik, et al., Science 354 (2016) 92–95. Crossref
(28). S.Y. Lien, P.J. Lai, W.R. Chen, C.H. Liu, et al., Crystals 12 (2022). Crossref
(29). S. Rühle, Solar Energy 130 (2016) 139–147. Crossref
(30). H. Chen, M. Li, B. Wang, S. Ming, et al., J. Alloy. Compd. 862 (2021) 158442. Crossref
(31). P. Cottingham, R.L. Brutchey, Chem. Mater. 28 (2016) 7574–7577. Crossref
(32). J. Zhou, F. Huang, H. Lin, Z. Lin, et al., J. Mater. Chem. C 4 (2016) 7601–7606. Crossref
(33). S.C. Shei, W.J. Chiang, S.J. Chang, Nanoscale Res. Lett. 10 (2015) 122. Crossref
(34). Z. Zhao, W. Xu, G. Pan, Y. Liu, et al., Mater. Res. Bull. 112 (2019) 142–146. Crossref
(35). M.R. Linaburg, E.T. McClure, J.D. Majher, P.M. Woodward, Chem. Mater. 29 (2017). Crossref
(36). D. Jia, J. Chen, X. Mei, W. Fan, et al., Energy Environ. Sci. 14 (2021) 4599–4609. Crossref
(37). D. Ghosh, M.Y. Ali, D.K. Chaudhary, S. Bhattacharyya, Solar Energy Mater. Sol. Cells 185 (2018) 28–35. Crossref
(38). S. Christodoulou, F. di Stasio, S. Pradhan, A. Stavrinadis, et al., J. Phys. Chem. C 122 (2018). 7621–7626. Crossref
(39). D. Ghosh, Y.M. Ali, A. Ghosh, A. Mandal, et al., J. Phys. Chem. C 125 (2021) 5485–5493. Crossref
(40). L. Hu, Q. Zhao, S. Huang, J. Zheng, et al., Nat. Commun. 12 (2021) 466. Crossref
(41). J. Khan, X. Zhang, J. Yuan, Y. Wang, et al., ACS Energy Lett. 5 (2020) 3322–3329. Crossref
(42). D. Aidarkhanov, Z. Ren, C.K. Lim, Z. Yelzhanova, et al., Solar Energy Mater. Sol. Cells 215 (2020) 110648. Crossref
(43). S. Akin, Y. Altintas, E. Mutlugun, S. Sonmezoglu, Nano Energy 60 (2019) 557–566. Crossref
(44). F. Cheng, R. He, S. Nie, C. Zhang, et al., J. Am. Chem. Soc. 143 (2021) 5855–5866. Crossref
Downloads
Published
How to Cite
Issue
Section
License
You are free to: Share — copy and redistribute the material in any medium or format. Adapt — remix, transform, and build upon the material for any purpose, even commercially.
Eurasian Chemico-Technological Journal applies a Creative Commons Attribution 4.0 International License to articles and other works we publish.
Subject to the acceptance of the Article for publication in the Eurasian Chemico-Technological Journal, the Author(s) agrees to grant Eurasian Chemico-Technological Journal permission to publish the unpublished and original Article and all associated supplemental material under the Creative Commons Attribution 4.0 International license (CC BY 4.0).
Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.